$ hdiutil makehybrid -iso -joliet -o Documents/tools/dest.iso /Volumes/source
So, all things equal, dd should be your best bet. Since dd is both fast and efficient. To use dd you'll have to check where your (dv|c)d is mounted.
$ diskutil list
/dev/disk0 (internal, physical):
#: TYPE NAME SIZE IDENTIFIER
0: GUID_partition_scheme *500.1 GB disk0
1: EFI EFI 209.7 MB disk0s1
2: Apple_CoreStorage Macintosh HD 499.2 GB disk0s2
3: Apple_Boot Recovery HD 650.0 MB disk0s3
/dev/disk1 (internal, virtual):
#: TYPE NAME SIZE IDENTIFIER
0: Apple_HFS Macintosh HD +498.9 GB disk1
Logical Volume on disk0s2
71E61617-FD0B-4FFA-A432-4FE2737C217D
Unlocked Encrypted
/dev/disk2 (disk image):
#: TYPE NAME SIZE IDENTIFIER
0: firefox_cache +596.7 MB disk2
/dev/disk4 (internal, physical):
#: TYPE NAME SIZE IDENTIFIER
0: CD_partition_scheme *861.7 MB disk4
1: CD_ROM_Mode_1 Hacking LiveCD 750.3 MB disk4s0
Looking at the CD entry, you'll want to create a binary copy of the disk4s0 image since this is the packed iso file. The other disk4 is the mounted and unpacked file system.
Before creating a copy you'll need to unmount the disk, so you can use it.
$ sudo diskutil umount /dev/disk4s0
Next, generate an ISO image with dd:$ sudo dd if=/dev/disk4s0 of=my.iso bs=2048 conv=sync,notrunc
Sudo is needed to access the 'real' disk iso. Once the disk image has been generated, check if it can boot with virtualbox.
If you wish to create a bootable CD using dd, just reverse the command, by using the iso ad if and the drive as of, check this guide if you're in doubt. Remember to chown and chmod the image if you wish others that root can use it.
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